J/A+A/549/A128    Singly deuterated isotopologues of formamide (Kutsenko+, 2013)

The extended spectroscopic database for deuterated species of formamide up to 1THz. Kutsenko A.S., Motiyenko R. A., Margules L., Guillemin J.-C. <Astron. Astrophys. 549, A128 (2013)> =2013A&A...549A.128K 2013A&A...549A.128K
ADC_Keywords: Atomic physics Keywords: ISM: molecules - molecular data - submillimeter: ISM - line: identification Abstract: Formamide (HCONH2) is the simplest molecule with a peptide bond detected in the interstellar medium. One of the keys for understanding the mechanisms for forming formamide in massive hot cores is the comparison of the relative abundances of its deuterated isotopologues. No deuterated species of formamide have been detected to date mostly owing to the lack of laboratory spectral data, which is limited by cm-wave measurements up to 40GHz. Therefore, we decided to extend the measurements and the analysis of the rotational spectra of deuterated isotopologues of formamide into terahertz range. We measured the rotational spectra of deuterated formamide in the frequency range 150-950GHz using the Lille fast-scan and solid-state source spectrometers. The ground vibrational states of 4 different isotopologues of formamide, DCONH2, cis-HCONHD, trans-HCONHD, and HCOND2 were assigned and analysed. The sets of the rotational and centrifugal distortion constants we obtained allow us to calculate accurate predictions of the transition frequencies for deuterated formamide in the frequency range above 1THz and at least for J<65 and Ka<25. Description: We provide a table with rotational transitions of the three singly deuterated isotopologues of formamide. The table contains line assignments, observed frequencies, residuals of the fits using A-reduction of the Watson's Hamiltonian and accuracy of frequency measurement. The quantum number F is indicated only for the transitions with resolved or partially resolved hyperfine structure. File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file table2.dat 78 8365 Assigned rotational transitions of the ground states of the studied singly deuterated isotopologues of formamide (HCONH2) -------------------------------------------------------------------------------- See also: J/A+A/493/565 : Deuterated and 15N ethyl cyanides (Margules+, 2009) J/A+A/538/A51 : Rotational spectrum of CH3CH(NH2)CN (Mollendal+, 2012) J/A+A/538/A119 : 18O-methyl formate (HCO18OCH3) spectrum (Tercero+ 2012) J/A+A/540/A51 : Submm spectrum of deuterated glycolaldehydes (Bouchez+, 2012) J/A+A/543/A46 : Submillimeter spectrum of HCOOCD2H (Coudert+, 2012) J/A+A/543/A135 : New analysis of 13C-CH3CH2CN up to 1THz (Richard+, 2012) J/A+A/544/A82 : Rotational spectroscopy of diisocyanomethane (Motiyenko+ 2012) J/A+A/548/A71 : Spectroscopy and ISM detection of formamide (Motiyenko+, 2012) Byte-by-byte Description of file: table2.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1- 9 A9 --- Species Isotopic species of formamide: DCONH2, c-HCONHD (cis), or t-HCONHD (trans) 11- 12 I2 --- J" Upper J quantum number 14- 15 I2 --- Ka" Upper Ka (rotational) quantum number 17- 18 I2 --- Kc" Upper Kc (rotational) quantum number 20- 21 I2 --- F" Upper F (hyperfine) quantum number 24- 25 I2 --- J' Lower J quantum number 27- 28 I2 --- Ka Lower Ka (rotational) quantum number 30- 31 I2 --- Kc' Lower Kc (rotational) quantum number 33- 34 I2 --- F' Lower F (hyperfine) quantum number 37- 48 F12.4 MHz Freq Observed transition frequency 51- 57 F7.4 MHz O-C Individual residuals of the fit 60- 64 F5.3 MHz unc Measurement uncertainty 67- 73 F7.4 MHz O-Cb ? Residuals of the blended components 75- 78 F4.2 --- Irel ? Relative intensity for blended line components -------------------------------------------------------------------------------- Acknowledgements: Roman Motiyenko, motienko(at)univ-lille1.fr
(End) Roman Motiyenko [PhLAM, Lille 1], Patricia Vannier [CDS] 29-Nov-2012
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