J/A+A/588/L8        Protonated formaldehyde in L1689B           (Bacmann+, 2016)

Detection of protonated formaldehyde in the prestellar core L1689B. Bacmann A., Garcia-Garcia E., Faure A. <Astron. Astrophys. 588, L8 (2016)> =2016A&A...588L...8B 2016A&A...588L...8B (SIMBAD/NED BibCode)
ADC_Keywords: Interstellar medium ; Spectroscopy Keywords: ISM: molecules - line: identification - ISM: abundances Abstract: Complex organic molecules (COMs) are detected in many regions of the interstellar medium, including prestellar cores. However, their formation mechanisms in cold (∼10K) cores remain to this date poorly understood. The formyl radical HCO is an important candidate precursor for several O-bearing terrestrial COMs in cores, as an abundant building block of many of these molecules. Several chemical routes have been proposed to account for its formation, both on grain surfaces, as an incompletely hydrogenated product of H addition to frozen-out CO molecules, or in the gas phase, either the product of the reaction between H2CO and a radical, or as a product of dissociative recombination of protonated formaldehyde H2COH+. The detection and abundance determination of H2COH+, if present, could provide clues as to whether this latter scenario might apply. We searched for protonated formaldehyde H2COH+ in the prestellar core L1689B using the IRAM 30m telescope. The H2COH+ ion is unambiguously detected, for the first time in a cold (∼10K) source. The derived abundance agrees with a scenario in which the formation of H2COH+ results from the protonation of formaldehyde. We use this abundance value to constrain the branching ratio of the dissociative recombination of H2COH+ towards the HCO channel to ∼10-30%. This value could however be smaller if HCO can be efficiently formed from gas-phase neutral- neutral reactions, and we stress the need for laboratory measurements of the rate constants of these reactions at 10K. Given the experimental difficulties in measuring branching ratios experimentally, observations can bring valuable constraints on these values, and provide a useful input for chemical networks. Description: Line parameters for the 4 H2COH+ transitions observed in the source L1689B. The frequency of the observed transition, the rms in the spectrum, the peak main beam temperature, the linewidth, the error on the linewidth, the line integrated intensity and the error on the integrated line intensity are given. The peak main beam temperature, linewidth and the integrated intensity were derived by Gaussian fitting of the spectra. The corresponding reduced (folded and baseline-subtracted) spectrum is given in antenna temperature units Ta*. Objects: ---------------------------------------------- RA (2000) DE Designation(s) ---------------------------------------------- 16 34 42.1 -24 36 11 L1689B = LDN 1689B ---------------------------------------------- File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file table2.dat 71 4 Line parameters for H2COH+ transitions sp/* . 4 Individual H2COH+ spectra -------------------------------------------------------------------------------- See Also: J/A+A/547/A33 : Chemical reactions for a deuteration network (Vastel+, 2012) J/A+A/587/A130 : HCO and CH3O in prestellar cores (Bacmann+, 2016) Byte-by-byte Description of file: table2.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1- 9 F9.2 MHz Freq Frequency of the transition 13- 15 F3.1 mK rms rms noise in spectrum 19- 21 I3 mK Tmb ?=- Line peak intensity, Tmb 26- 29 F4.2 km/s dv ?=- Linewidth 33- 36 F4.2 km/s e_dv ?=- Error on linewidth 40 A1 --- l_Int Limit flag on intensity 41- 46 F6.4 K.km/s Int Integrated intensity 49- 54 F6.4 K.km/s e_Int ?=- Error on integrated intensity 58- 71 A14 --- FileName Name of corresponding spectrum file in subdirectory sp -------------------------------------------------------------------------------- Byte-by-byte Description of file: sp/* -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 4- 13 F10.3 MHz Freq Frequency 19- 30 E12.5 K Int Intensity in Ta* unit -------------------------------------------------------------------------------- Acknowledgements: Aurore Bacmann, aurore.bacmann(at)univ-grenoble-alpes.fr
(End) Aurore Bacmann [IPAG], Patricia Vannier [CDS] 07-Mar-2016
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