J/A+A/619/A67   Rotational spectrum of methoxyacetaldehyde (Kolesnikova+, 2018)

Laboratory rotational spectrum and astronomical search for methoxyacetaldehyde. Kolesnikova L., Pena I., Alonso E.R., Tercero B., Cernicharo J., Mata S., Alonso J.L. <Astron. Astrophys. 619, A67 (2018)> =2018A&A...619A..67K 2018A&A...619A..67K (SIMBAD/NED BibCode)
ADC_Keywords: Interstellar medium ; Spectroscopy ; Atomic physics Keywords: astrochemistry - ISM: molecules - line: identification - astronomical databases: miscellaneous - Abstract: Methoxyacetaldehyde belongs to a group of structural isomers with the general formula C3H6O2, of which methyl acetate and ethyl formate are known interstellar molecules. Rotational data available for methoxyacetaldehyde are limited to 40GHz, which makes predictions at higher frequencies rather uncertain. The aim of this work is to provide accurate experimental frequencies of methoxyacetaldehyde in the millimeter-wave region to support its detection in the interstellar medium. The rotational spectrum of methoxyacetaldehyde was recorded at room-temperature from 75 to 120GHz and from 170 to 310GHz using the millimeter-wave spectrometer in Valladolid. Additional measurements were also performed at conditions of supersonic expansion from 6 to 18GHz. The assigned rotational transitions were analyzed using the S-reduced semirigid-rotor Hamiltonian. We newly assigned over 1000 lines for the most stable conformer of methoxyacetaldehyde in its ground state and five lowest excited vibrational states, and precise sets of spectroscopic constants were obtained. We searched for spectral features of methoxyacetaldehyde in the high-mass star-forming regions Orion KL and Sagittarius B2, as well as in the cold dark cloud Barnard 1 (B1-b). No lines belonging to methoxyacetaldehyde were detected above the detection limit of our data. We provide upper limits to the methoxyacetaldehyde colum density in these sources. Description: Observed rotational transitions of methoxyacetaldehyde in the ground state and excited vibrational states. File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file table4.dat 126 1353 Fitted rotational transitions of methoxyacetaldehyde in the ground state and excited vibrational states -------------------------------------------------------------------------------- See also: J/A+A/577/A91 : Millimeter wave spectrum of vinyl acetate (Kolesnikova+, 2015) J/A+A/591/A75 : Millimeter wave spectrum of methyl cyanate (Kolesnikova+ 2016) J/ApJ/832/42 : Rotational spectrum of vinyl formate (Alonso+, 2016) J/ApJS/229/26 : Rotational spectra of aminoacetonitrile (Kolesnikova+, 2017) J/ApJS/233/24 : Iso-propyl cyanide rotational study (Kolesnikova+, 2017) J/A+A/609/A24 : Rotational spectrum of methoxyamine (Kolesnikova+, 2018) J/A+A/616/A173 : Rotational spectrum of ethyl isocyanate (Kolesnikova+, 2018) Byte-by-byte Description of file: table4.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1- 3 I3 --- J' Upper state J quantum number 4- 6 I3 --- Ka' Upper state Ka quantum number 7- 9 I3 --- Kc' Upper state Kc quantum number 10- 12 I3 --- J" Lower state J quantum number 13- 15 I3 --- Ka" Lower state Ka quantum number 16- 18 I3 --- Kc" Lower state Kc quantum number 23- 33 F11.4 MHz FreqObs Observed transition frequency 36- 42 F7.4 MHz O-C Observed minus calculated frequency 45- 50 F6.4 MHz e_FreqObs Experimental uncertainty 53- 59 F7.4 MHz (O-C)b ? Observed minus calculated frequency for blends 61- 64 F4.2 --- wb ? Weight of the components of the blends 68-126 A59 --- Notes Vibrational state and the source of the data (1) -------------------------------------------------------------------------------- Note (1): Hirono et al., 1987, J. Mol. Struc., 162, 359. -------------------------------------------------------------------------------- Acknowledgements: Lucie Kolesnikova, lucie.kolesnikova(at)uva.es
(End) Lucie Kolesnikova [GEM, UVa, Spain], Patricia Vannier [CDS] 07-Nov-2018
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