J/A+A/675/A69       First detection of CD toward IRAS 16293-2422  (Jacob+, 2023)

First detection of deuterated methylidyne (CD) in the interstellar medium. Jacob A.M., Menten K.M., Wyrowski F., Sipila O. <Astron. Astrophys. 675, A69 (2023)> =2023A&A...675A..69J 2023A&A...675A..69J (SIMBAD/NED BibCode)
ADC_Keywords: Molecular clouds ; Infrared sources ; Spectroscopy Keywords: astrochemistry - ISM: molecules - ISM: individual objects: IRAS 16293-2422 - line: identification - molecular data Abstract: While the abundance of elemental deuterium is relatively low (D/H ∼ a few x 10-5), orders of magnitude higher D/H abundance ratios have been found for many interstellar molecules, enhanced by deuterium fractionation. In cold molecular clouds (T<20K) deuterium fractionation is driven by the H2D+ ion, whereas at higher temperatures (T>20-30K) gas-phase deuteration is controlled by reactions with CH2D+ and C2HD+. While the role of H2D+ in driving cold interstellar deuterium chemistry is well understood, thanks to observational constraints from direct measurements of H2D+, deuteration stemming from CH2D+ is far less understood, as a result of the absence of direct observational constraints of its key ions. Therefore, making use of chemical surrogates is imperative in order to explore deuterium chemistry at intermediate temperatures. Formed at an early stage of ion-molecule chemistry directly from the dissociative recombination of CH3+ (CH2D+), CH (CD) is an ideal tracer for investigating deuterium substitution initiated by reactions with CH2D+. This paper reports the first detection of CD in the interstellar medium (ISM), carried out using the APEX 12m telescope towards the widely studied low-mass protostellar system IRAS 16293-2422. Observed in absorption toward the envelope of the central protostar, the D/H ratio derived from the column densities of CD and CH is found to be 0.016±0.003. This is an order of magnitude lower than the values found for %that derived using other small molecules like C2H and H2CO observed in emission but whose formation, which is similar to that of CH, is also initiated via pathways involving warm deuterium chemistry. Gas-phase chemical models reproducing the CD/CH abundance ratio suggest that it reflects 'warm deuterium chemistry' (which ensues in moderately warm conditions of the ISM) and illustrates the potential use of the CD/CH ratio in constraining the gas temperatures of the envelope gas clouds it probes. Description: Observations of the N=1, J=3/2-1/2 hyperfine structure splitting transitions of CD near 440GHz were performed in June 2021 and April and June 2022 using the high-frequency module of the new version of the First Light APEX Submillimetre Heterodyne Receiver, nFLASH460, on the APEX 12m telescope under the project id:M9530C_107. We report the detect towards IRAS 16293-2422 as well as the non-detection towards star-forming regions SgrB2M, G34.26+0.15 and W49N. In addition to the results of the CD observations described above, we use complementary Herschel/HIFI archival data of CH at 532/526 GHz published in Bottinelli et al. (2014MNRAS.441.1964B 2014MNRAS.441.1964B). Furthermore toward W49N we also report the non-detection of the N=2-1, J=3/2-1/2 hyperfine structure splitting lines of CD near 1325GHz using the 4GREAT instrument on SOFIA under project id: 83_0701. Objects: ---------------------------------------------------------------------- RA (2000) DE Designation(s) ---------------------------------------------------------------------- 16 32 22.56 -24 28 31.8 IRAS 16293-2422 = JCMTSE J163222.8-242837 ---------------------------------------------------------------------- File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file list.dat 165 2 List of fits spectra fits/* . 2 Individual fits spectra -------------------------------------------------------------------------------- Byte-by-byte Description of file: list.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1- 9 F9.5 deg RAdeg Right Ascension of center (J2000) 10- 18 F9.5 deg DEdeg Declination of center (J2000) 20- 22 I3 --- Nx Number of pixels along X-axis 24- 46 A23 "datime" Obs.date Observation date 48- 59 E12.6 Hz bFreq Lower value of frequency interval 61- 71 E11.6 Hz BFreq Upper value of frequency interval 73- 78 I6 Hz dFreq Frequency resolution 80- 82 F3.1 km/s vlsr Source LSR velocity 84- 87 F4.2 K Tc Main-beam brightness continuum temperature at 440GHz 89- 94 A6 --- Parity Parity of the N=1, J=3/2-1/2 transitions of CD 96 I1 Kibyte size Size of FITS file 98-121 A24 --- FileName Name of FITS file, in subdirectory fits 123-165 A43 --- Title Title of the FITS file -------------------------------------------------------------------------------- Acknowledgements: Arshia Maria Jaocb, ajacob51(at)jhu.edu References: Bottinelli et al., 2014MNRAS.441.1964B 2014MNRAS.441.1964B, CH in absorption in IRAS 16293-242 Jacob et al., 2020A&A...640A.125J 2020A&A...640A.125J, First detection of 13CH in the interstellar medium
(End) Patricia Vannier [CDS] 12-May-2023
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