J/A+A/681/L19       HCNH+ abundance in cold dense clouds            (Bop+, 2024)

HCNH+ abundance in cold dense clouds based on the first hyperfine resolved rate coefficients. Bop T.C., Agundez M., Cernicharo J., Lefloch B., Lique F. <Astron. Astrophys. 681, L19 (2024)> =2024A&A...681L..19B 2024A&A...681L..19B (SIMBAD/NED BibCode)
ADC_Keywords: Atomic physics Keywords: molecular data - molecular processes - radiative transfer - scattering - ISM : abundances - ISM: molecules Abstract: The protonated form of hydrogen cyanide, HCNH+, holds significant importance in astrochemistry, serving as an intermediate species in ion-neutral reactions occurring in the cold molecular clouds. Although it plays a crucial role in the chemistry of HCN and HNC, the excitation rate coefficients of this molecular cation by the dominant interstellar colliders have not been thoroughly investigated, leading to limitations in radiative transfer models use to derive its abundance. We present here the first hyperfine-resolved excitation rate coefficients for HCNH+ induced by collisions with both He and H2 at low temperatures, addressing a crucial requirement for precise modeling of HCNH+ abundance in typical cold dense molecular clouds. Using non-local thermodynamic equilibrium (LTE) radiative transfer calculations, we reproduce fairly well the 1-->0 and 2-->1 observational spectra of HCNH+ and derive updated molecular column densities. For the TMC-1 molecular cloud, the new HCNH+ abundance is twice larger than suggested by previous LTE modeling, whereas the column density of this molecular cation is improved only by 10% in the case of the L483 proto-star. The factor of 2 in the case of TMC-1 most likely arises from an error in the early analysis of observational spectra rather than an effect of the LTE assumption, given that the HCNH+ lines are predominantly thermalized at densities higher than 2x104cm-3. For multiline studies of clouds of moderate density, we strongly recommend to use the collisional rate coefficients reported in this work. Description: The first hyperfine resolved rate coefficients of HCNH+ induced by collision with H2 and He was derived using the most accurate recoupling method based on nuclear spin-independent scattering matrices calculated by mean of the close-coupling quantum mechanical approach. The data are in cm-3.s-1. File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file hcnhp-el.dat 34 25 Rotational energy levels of HCNH+ hcnhp-h2.dat 120 324 HFS rates due to collision with H2 hcnhp-he.dat 120 324 HFS rates due to collision with He -------------------------------------------------------------------------------- Byte-by-byte Description of file: hcnhp-el.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 4- 5 I2 --- Level [1/25] Level identification number 10- 19 F10.7 --- E Energy 24- 27 F4.1 --- Weith Weight 32- 34 A3 --- J-F J and F transition (J_F) -------------------------------------------------------------------------------- Byte-by-byte Description of file: hcnhp-h2.dat hcnhp-he.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 6- 8 I3 --- Trans Trasnsition identification number 15- 16 I2 --- Up [1/25] Upper level number 23- 24 I2 --- Low [1/25] Lower level number 29- 40 E12.7 cm-3.s-1 RCT5 First hyperfine resolved rate coefficient for T=5.0K 45- 56 E12.7 cm-3.s-1 RCT10 First hyperfine resolved rate coefficient for T=10.0K 61- 72 E12.7 cm-3.s-1 RCT15 First hyperfine resolved rate coefficient for T=15.0K 77- 88 E12.7 cm-3.s-1 RCT20 First hyperfine resolved rate coefficient for T=20.0K 93-104 E12.7 cm-3.s-1 RCT25 First hyperfine resolved rate coefficient for T=25.0K 109-120 E12.7 cm-3.s-1 RCT30 First hyperfine resolved rate coefficient for T=30.0K -------------------------------------------------------------------------------- Acknowledgements: Tidiane Cheikh Bop, cheikhtidiane.bop(at)ucad.edu.sn
(End) Patricia Vannier [CDS] 06-Jan-2024
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