J/ApJ/909/8          Molybdenum isotopes in meteorites          (Stephan+, 2021)

Molybdenum isotope dichotomy in meteorites caused by s-process variability. Stephan T., Davis A.M. <Astrophys. J., 909, 8 (2021)> =2021ApJ...909....8S 2021ApJ...909....8S
ADC_Keywords: Meteorites; Abundances Keywords: Meteorites ; Circumstellar grains ; S-process ; R-process ; P-process ; Nucleosynthesis ; Solar system formation ; Isotopic abundances Abstract: Molybdenum isotopes measured in most individual presolar silicon carbide grains are dominated by s-process contributions from the helium intershells of asymptotic giant branch (AGB) stars. The much smaller isotopic variations in molybdenum in meteorites and their components are largely controlled by s-process enrichments or depletions relative to terrestrial composition but lie along two parallel s-process mixing lines separated by what has been suggested to be an r-process contribution. The two mixing lines are populated by carbonaceous-chondrite- and noncarbonaceous-chondrite-related meteorites (CC and NC groups, respectively). We have compared molybdenum isotopic data for presolar grains with those from meteorites and renormalized the meteorite data in a way that is consistent with s-, r-, and p-process contributions observed in presolar SiC grains. The results indicate that (1) there seems to be a fixed ratio between p- and r-process contributions in all data, (2) the dichotomy in molybdenum isotopes between the CC and NC groups can be explained by variations in the isotope makeup of the s-process contribution to the meteoritic samples, (3) this variability is similar to the variations in s-process molybdenum from different AGB stars deduced from presolar grain analyses, and (4) the larger range of isotopic compositions found in refractory inclusions is also consistent with s-process isotope variability. File Summary: -------------------------------------------------------------------------------- FileName Lrecl Records Explanations -------------------------------------------------------------------------------- ReadMe 80 . This file tablea1.dat 153 269 Meteorite molybdenum isotope data renormalized to ε98Mo9692Mo96=0.256 -------------------------------------------------------------------------------- See also: J/MNRAS/418/284 : s-process in low-metallicity stars. II. (Bisterzo+, 2011) J/ApJ/743/L23 : 48Ca heterogeneity in differentiated meteorites (Chen+, 2011) J/ApJ/758/45 : Isotopic Sr abundances in meteorites (Moynier+, 2012) J/ApJ/758/59 : Nickel isotopes in meteorites (Steele+, 2012) J/ApJ/787/10 : Solar s-process contributions with GCE model (Bisterzo+, 2014) J/ApJ/854/18 : Nucleosynthesis of p nuclides (Travaglio+, 2018) Byte-by-byte Description of file: tablea1.dat -------------------------------------------------------------------------------- Bytes Format Units Label Explanations -------------------------------------------------------------------------------- 1 I1 --- Group [1/3] Meteorite group (1) 3- 25 A23 --- Subgroup Subgroup 27- 46 A20 --- Type Type (2) 48- 72 A25 --- Sample Meteorite/Sample (2) 74- 79 F6.2 --- eps92Mo96 [-52.03/19.98] Molybdenum-92 isotopic data 81- 84 F4.2 --- e_eps92Mo96 [0.02/2.1] 1σ uncertainty in eps92Mo96 86- 91 F6.2 --- eps94Mo96 [-50.92/18.92] Molybdenum-94 isotopic data 93- 96 F4.2 --- e_eps94Mo96 [0.02/1.9] 1σ uncertainty in eps94Mo96 98- 103 F6.2 --- eps95Mo96 [-31.47/12.66] Molybdenum-95 isotopic data 105- 108 F4.2 --- e_eps95Mo96 [0.01/1.1] 1σ uncertainty in eps95Mo96 110- 115 F6.2 --- eps97Mo96 [-27.43/10.35] Molybdenum-97 isotopic data 117- 120 F4.2 --- e_eps97Mo96 [0/0.7] 1σ uncertainty in eps97Mo96 122- 127 F6.2 --- eps98Mo96 [-13.3/5.11] Molybdenum-98 isotopic data 129- 132 F4.2 --- e_eps98Mo96 [0/0.5] 1σ uncertainty in eps98Mo96 134- 139 F6.2 --- eps100Mo96 [-51.73/19.8] Molybdenum-100 isotopic data 141- 144 F4.2 --- e_eps100Mo96 [0.01/2.2] 1σ uncertainty in eps100Mo96 146- 151 A6 --- Ref Reference (3) 153 A1 --- Notes Notes (4) -------------------------------------------------------------------------------- Note (1): Meteorite grouping codes as follows: 1 = Carbonaceous-Chondrite-Related (CC) Meteorites; 2 = Noncarbonaceous-Chondrite-Related (NC) Meteorites; 3 = Calcium-aluminum-rich inclusions (CAIs). Note (2): Meteorite names and types, which are in some cases different from those in the original publications cited here, are given according to the Meteoritical Bulletin Database (http://www.lpi.usra.edu/meteor/). For detailed sample descriptions, please refer to the original literature. CAIs are subdivided into unfractionated and fractionated groups according to Brennecka+ (2013PNAS..11017241B 2013PNAS..11017241B). Uncertainties are 1σ. Note (3): References as follows: Dau02a = Dauphas et al. (2002ApJ...565..640D 2002ApJ...565..640D); Dau02b = Dauphas et al. (2002ApJ...569L.139D 2002ApJ...569L.139D); Bur11 = Burkhardt et al. (2011E&PSL.312..390B 2011E&PSL.312..390B); Bur12 = Burkhardt et al. (2012E&PSL.357..298B 2012E&PSL.357..298B); Bre13 = Brennecka et al. (2013PNAS..11017241B 2013PNAS..11017241B); Bur14 = Burkhardt et al. (2014E&PSL.391..201B 2014E&PSL.391..201B); Bud16 = Budde et al. (2016E&PSL.454..293B 2016E&PSL.454..293B); Kru17 = Kruijer et al. (2017PNAS..114.6712K 2017PNAS..114.6712K); Ren17 = Render et al. (2017, Geochem. Perspect. Lett. 3, 170); Wor17 = Worsham et al. (2017E&PSL.467..157W 2017E&PSL.467..157W); Ber18 = Bermingham et al. (2018E&PSL.487..221B 2018E&PSL.487..221B); Sho18 = Shollenberger et al. (2018GeCoA.228...62S 2018GeCoA.228...62S); Bud18 = Budde et al. (2018GeCoA.222..284B 2018GeCoA.222..284B); Bud19 = Budde et al. (2019NatAs...3..736B 2019NatAs...3..736B); Wor19 = Worsham et al. (2019E&PSL.521..103W 2019E&PSL.521..103W); Yok19 = Yokoyama et al. (2019ApJ...883...62Y 2019ApJ...883...62Y); Bre20 = Brennecka et al. (2020Sci...370..837B 2020Sci...370..837B); Hop20 = Hopp et al. (2020E&PSL.53416065H 2020E&PSL.53416065H); Spi20 = Spitzer et al. (2020ApJ...898L...2S 2020ApJ...898L...2S). Note (4): Notes on individual values as follows: a = Platinum data for CRE correction were taken from Kruijer+ (2017PNAS..114.6712K 2017PNAS..114.6712K); b = In the original publication (Render+ 2017, Geochem. Perspect. Lett. 3, 170), EET 87746 (EH4 enstatite chondrite) was incorrectly reported as EET 87747 (EH4), which would instead be a CR2 carbonaceous chondrite; c = Sombrerete was initially attributed to the CC meteorite group (Worsham+ 2017E&PSL.467..157W 2017E&PSL.467..157W) but is here counted as a NC meteorite like all other IAB iron meteorites. Due to the large errors of this single analysis, this has no significant impact on any results or conclusions; d = CAI types for CAIs analyzed by Brennecka+ (2013PNAS..11017241B 2013PNAS..11017241B) were provided by Shollenberger+ (2018GeCoA.228...62S 2018GeCoA.228...62S). -------------------------------------------------------------------------------- History: From electronic version of the journal
(End) Prepared by [AAS], Emmanuelle Perret [CDS] 05-Aug-2022
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